Abstract: Six terpeniods were isolated from the EtOH extracts of Curculigo orchioides by a series separation method. They were identified as (3S, 5R, 6S, 7E, 9R)-megatigma-7-ene-3,5,6,9-tetrol (1), actinidioionoside (2), (6S, 9R)-roseoside (3), (−)-angelicoidenol 2-o-β-D-lucopyranoside (4), (−)-angelicoidenol-2-o-β-apiofuranosyl-(1→6)-β-D-glucopyranoside (5) and tetillapyrone (7R, 9S, 10R)-3-methyl-5-(4-hydroxyl-5-hydroxylmethyltetrahydrofuryl)-6-hydroxypyran-2-one (6) through manifold spectroscopic means (HRESIMS and NMR). This was the first time that reported the terpeniods from Curculigo orchioides and enriched the chemical constituents of this species.